Wohl-Ziegler reaction

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The Wohl-Ziegler reaction[1][2] is a chemical reaction that involves the allylic or benzylic bromination of hydrocarbons using an N-bromoimide and a radical initiator.[3]

The Wohl-Ziegler reaction
The Wohl-Ziegler reaction

Best yields are achieved with N-bromosuccinimide in carbon tetrachloride solvent.

Several reviews have been published.[4][5]

In a typical setup a a stoichiometric amount of N-bromosuccinimide solution and a small quantity of initiator are added to a solution of the substrate in CCl4, and the reaction mixture is stirred and heated to the boiling point. Initiation of the reaction is indicated by more vigorous boiling; sometimes the heat source may need to be removed. Once all N-bromosuccinimide (which is denser than the solvent) has been converted to succinimide (which floats on top) the reaction has finished.

References

  1. Wohl, A. Ber. 1919, 52, 51.
  2. Ziegler, K.; et al. Ann. 1942, 551, 30.
  3. Template:OrgSynth
  4. C. Djerassi (1948). "Brominations with N-Bromosuccinimide and Related Compounds. The Wohl-Ziegler Reaction". Chem. Rev. 43 (2): 271–317. doi:10.1021/cr60135a004.
  5. Horner, L.; Winkelman, E. M.; Angew. Chem. 1959, 71, 349. (Review)


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